Wiley能源催化領域最新進展 雙金屬MOF、界面電子調控、合金設計、雜原子摻雜納米線、核殼結構01. 雙金屬MOF作為高效氧電催化劑開發不含貴金屬的雙功能氧電催化劑對一些關鍵的能源轉換和存儲系統具有重要意義，但仍然存在巨大挑戰。在此，新加坡南洋理工大學樓雄文教授課題組開發了一種轉化方法，以在多-通道碳纖維（MCCF）上生長NiMn-基雙金屬-有機框架（NiMn-MOF）納米片的潛在雙功能氧電催化劑。由于活性NiMn-MOF納米片及其與高度導電的MCCF載體緊密連接，所獲得的MCCF/NiMn-MOFs表現出可與商用Pt/C電催化劑相媲美的氧氣還原反應（ORR）電催化性能和優異的氧氣析出反應（OER）性能（基于基準RuO2電催化劑）。X-射線吸收精細結構（XAFS）譜和密度泛函理論（DFT）計算表明，MCCF/NiMn-MOFs中相鄰Ni和Mn節點強的協同作用有效促進了關鍵*O和*OOH中間體的熱力學，

幸運之星電子遊藝場

從而實現快速的ORR和OER動力學。原文鏈接：https://onlinelibrary.wiley.com/doi/abs/10.1002/anie.20200812902. 調節界面電子耦合以進行HER操縱界面電子耦合的能力是實現催化劑按需功能的關鍵。在此，中國科學技術大學錢逸泰/王功名/劉曉靜團隊和國家同步輻射實驗室朱俊發/鄭旭升團隊合作，證明了可以通過空位-介導的軌道操縱來有效地調節Fe2N的電子耦合以進行氫氣析出反應（HER）催化。非原位精修結構分析表明，Fe2N的電子和配位態可以很好地被氮空位所操縱，

土耳其強震

這與催化活性具有顯著的相關性。理論研究進一步表明，氮的空位可以唯一地控制活性位的軌道取向，以調節電子耦合，

全球即時比分網

從而有利于表面吸附能力。這項工作闡明了對真實系統中催化機理的理解，

上海初中生發現教科書用圖有誤

並可能有助于徹底改變目前用于HER的催化劑設計。原文鏈接：https://onlinelibrary.wiley.com/doi/abs/10.1002/adma.20190434603. 腐蝕與合金設計實現高效分解水由于清潔能源領域的不斷增長，

內蒙古司法廳原廳長徐呼和被查

Ni、Fe、Co、Cu（除稀土金屬外）是一些需求旺盛的關鍵材料。在此，韓國漢陽大學Sung Chul Yi課題組通過將廢舊輪胎的不鏽鋼絲（SSW）作為載體材料，以整合氫氣析出反應（HER）中的催化劑。此外，通過腐蝕設計的SSW被用作原位形成的自支撐堅固電極，以進行氧氣析出反應（OER）。通過SSW的表面腐蝕，內在的活性物質以Ni/FeOOH納米微晶的形式存在，

pk10開獎

其在1 M KOH中以287 mV低的過電勢（η500）能夠達到500 mA cm-2，

土耳其強震

顯示出有效的水氧化作用。類似地，具有MoNi4活性（合金）塗層的正極廢料SSW在η-200= 77 mV時催化HER，活化能低（Ea= 16.338 kJ mol-1）且具有150 h長的耐久性。甚至，當在5 M KOH、343 K的工業條件下使用時，這些電極可分別在η= 233 mV和η= 161 mV時產生1000 mA cm-2的高負極和正極電流密度，進一步證明該材料的活性。這項工作可能會激發研究人員探索和重新利用廢料中的高需求金屬，以解決清潔能源技術中的關鍵材料短缺問題。原文鏈接：https://onlinelibrary.wiley.com/doi/abs/10.1002/aenm.20190402004. 雜原子摻雜Co納米線有效分解水為了更好地分解水，必須迅速開發出具有高活性、長期穩定性和成本效益的高效催化劑。在這項工作中，韓國全北國立大學Joong Hee Lee/Duy Thanh Tran團隊制備了一種雙功能催化劑，其由一層薄的Mo，P-共摻雜Co層（約50 nm）和Co納米線（Co-Mo-P/CoNWs）網絡自組裝而成。為達到20 mA cm-2的電流響應，該催化劑對氫氣析出反應和氧氣析出反應可分別展現出0.08和0.27 V低的過電勢，並且在1.0 M KOH介質中具有長期穩定性。出色的性能進一步得到基于Co-Mo-P/CoNWs電解槽的證實，其僅需1.495 V的電池電壓就能達到10 mA cm-2，

幸運之星電子遊藝場

優于商用的（Pt/C + RuO2/C ）以及最近所報道的。普遍認為，

賓果賓果開獎號碼奧索樂透網

由Mo和P雙重摻雜引起的多活性中心以及增加的活性位點協同促進了氫氣和氧氣的析出性能。這種雜化材料為開發高效且具有成本效益的水分解催化劑開闢了新途徑。原文鏈接：https://onlinelibrary.wiley.com/doi/abs/10.1002/adfm.20200253305. 磷摻雜氮化鐵@氮摻雜碳納米片用于水分解提出一種新穎、經濟、安全的制備方法來設計高效的電催化劑至關重要。在此，濟南大學週偉家/劉宏/Xiaoyan Liu團隊通過原位衍生釀酒酵母（S. cerevisiae），將磷-摻雜的氮化鐵納米離子（被氮-摻雜碳納米片封裝）直接生長在泡沫鐵基底上（P-Fe3N@NC NSs/IF），其中的陰離子元素為S. cerevisiae中的C、N和P都替代了危險的CH4、NH3和H3P。N、P在S. cerevisiae中的擴散方式以及金屬和S. cerevisiae之間的接觸形式可影響高溫鍛燒過程中產物的組成和相。所獲得的P-Fe3N@NC NSs/IF表現出優異的電催化性能和耐久性，可用于氫氣析出反應和氧氣析出反應。理論計算證實，P-Fe3N的Fe位點是活性中心，並且N位點和P摻雜調節了氫氣結合強度以增強催化能力。此外，

食堂師傅貼結婚告示學生送祝福

由P-Fe3N@NC NSs/IF組裝成的兩電極電解槽僅需1.61 V的電壓即可達到10 mA cm-2的全解水效果，並具有出色的穩定性。基于S. cerevisiae的工藝為合成氮化物、碳化物、磷化物和電催化應用提供了一種可行的方法。原文鏈接：https://onlinelibrary.wiley.com/doi/abs/10.1002/smll.202001980 （本期作者：毛毛的維）Publications of Dr. Peijian Shi2009Shi錛 P.錛 Liu錛 J.錛 Yang錛 Z. 2009. Spatio-temporal point pattern analysis on Wenchuan strong earthquake. Earthquake Science 22: 231−2372010Shi錛 P.錛 Ge錛 F. 2010. A comparison of different thermal performance functions describing temperature-dependent development rates. Journal of Thermal Biology 35: 225−231Shi錛 P.錛Ge錛 F.錛 Men錛 X. 2010. How to compare the lower developmental thresholds. Environmental Entomology 39: 2033−2038時培建錛郭世權錛 楊清培錛 王兵錛 楊光耀錛 方凱. 毛竹的異質性空間點格局分析. 生態學報. 30(16): 4401−44072011 時培建錛 戈峰錛 楊清培. 棲息地永久性破壞的比例對物種多度穩定值影響的迭代算法. 生態學報. 31(15): 4327−4333Bonato錛 O.錛 Ikemoto錛 T.錛 Shi錛 P.錛 Ge錛 F.錛 Sun錛 Y.錛 Cao錛 H. 2011. Common-intersection hypothesis of development rate lines of ectotherms within a taxon revisited. Journal of Thermal Biology 36: 422−429 Sandhu錛 H. S.錛 Shi錛 P.錛 Kuang錛 X.錛 Xue錛 F.錛 Ge錛 F. 2011. Applications of the bootstrap to insect physiology. Florida Entomologist 94: 1036−1041 Shi錛 P.錛 Ikemoto錛 T.錛 Egami錛 C.錛 Sun錛 Y.錛 Ge錛 F. 2011. A modified program for estimating the parameters of the SSI model. Environmental Entomology 40: 462−469 Shi錛 P.錛 Ge錛 F.錛 Sun錛 Y.錛 Chen錛 C. 2011. A simple mode for describing the effect of temperature on insect developmental rate. Journal of Asia-Pacific Entomology 14: 15−20 2012 Kuang X.錛 Parajulee錛 M.N.錛 Shi錛 P.錛 Ge錛 F.錛 Xue錛 F. 2012. Testing the rate isomorphy hypothesis using five statistical methods. Insect Science 19: 121−128 Reddy錛 G.V.P.錛 Shi錛 P.錛 Mann錛 C.R. et al. 2012. Can a semiochemical-based trapping method diminish damage levels caused by Rhabdoscelus obscurus (Coleoptera: Curculionidae)? Annals of the Entomological Society of America 105: 693−700 Shi錛 P.錛 Li錛 B.-L.錛 Ge錛 F. 2012. Intrinsic optimum temperature of the diamondback moth and its ecological meaning. Environmental Entomology 41: 714−722 Shi錛 P.錛 Wang錛 B.錛 Ayres錛 M.P.錛 Ge錛 F.錛 Zhong錛 L.錛 Li錛 B.-L. 2012. Influence of temperature on the northern distribution limits of Scirpophaga incertulas Walker (Lepidoptera: Pyralidae) in China. Journal of Thermal Biology 37: 130−137 Shi錛 P.錛 Zhong錛 L.錛 Sandhu錛 H.S錛 Ge錛 F.錛 Xu錛 X.錛 Chen錛 W. 2012. Population decrease of Scirpophaga incertulas Walker (Lepidoptera Pyralidae) under climate warming. Ecology and Evolution 2: 58−64 2013 Chakraborty錛 A.錛 Shi錛 P.錛 Liu錛 Q.錛 Yang錛 Q.錛 Li錛 B. 2013. A commensal consumer-induced mediation effects on resource-consumer interactions. Proceedings of the National Academy of Sciences錛 India – Section B: Biological Sciences 83: 385−404 Ikemoto錛 T.錛 Kurahashi錛 I.錛 Shi錛 P.錛 2013. Confidence interval of intrinsic optimum temperature estimated by using thermodynamic SSI model. Insect Science 20: 420−428 Sandhu錛 H.S.錛 Shi錛 P.錛 Yang錛 Q. 2013. Intraspecific spatial niche differentiation: evidence from Phyllostachys edulis. Acta Ecologica Sinica 33: 287−292[毛竹的種瓤佔瀋環擲]Shi錛 P.錛 Men錛 X.錛 Sandhu錛 H.S.錛 Chakraborty錛 A.錛 Li錛 B.錛 Ouyang錛 F.錛 Sun錛 Y.錛 Ge錛 F. 2013. The "general" ontogenetic growth model is inapplicable to crop growth. Ecological Modelling 266: 1−9 Shi錛 P.錛 Sandhu錛 H.S.錛 Xiao錛 H. 2013. Logistic regression is a better method of analysis than linear regression of arcsine square root transformed proportional diapause data of Pieris melete (Lepidoptera: Pieridae). Florida Entomologist 96: 1183−1185 Shi錛 P.錛 Sandhu錛 H.S.錛 Ge錛 F. 2013. Could the intrinsic rate of increase represent the fitness in terrestrial ectotherms? Journal of Thermal Biology 38: 148−151 Wang錛 L.錛 Shi錛 P.錛 Chen錛 C.錛 Xue錛 F. 2013. Effect of temperature on the development of Laodelpha xstriatellus (Homoptera: Delphacidae). Journal of Economic Entomology 106: 107−114 Zhao錛 Z.錛 Shi錛 P. (共同第一作者)錛 Hui錛 C.錛 Ouyang錛 F.錛 Ge錛 F.錛 Li錛 B.-L. 2013. Solving the pitfalls of pitfall trapping: a two-circle method for density estimation of ground-dwelling arthropods. Methods in Ecology and Evolution 4: 865−871 Zhao錛 Z.錛 Shi錛 P.錛 Men錛 X.錛 Ouyang錛 F.錛 Ge錛 F. 2013. Effects of crop species richness on pest-natural enemy systems based on an experimental model system using a microlandscape. Science China Life Sciences 56: 758−766 2014 Ouyang錛 F.錛 Hui錛 C.錛 Ge錛 S.Y.錛 Men錛 X.Y.錛 Zhao錛 Z.H.錛 Shi錛 P.J.錛 Zhang錛 Y.S.錛 Li錛 B.L. 2014. Weakening density dependence from climate change and agricultural intensification triggers pest outbreaks: a 37-year observation of cotton bollworms. Ecology and Evolution 4: 3362−3374 Shi錛 P.錛 Ishikawa錛 T.錛 Sandhu錛 H.S.錛 Hui錛 C.錛 Chakraborty錛 A.錛 Jin錛 X.錛 Tachihara錛 K.錛 Li錛 B. 2014. On the 3/4-exponent von Bertalanffy equation for ontogenetic growth. Ecological Modelling 276: 23−28 Shi錛 P.錛 Hui錛 C.錛 Men錛 X.錛 Hui錛 C.錛 Zhao錛 Z.錛 Ouyang錛 F.錛 Cao錛 H.錛 Jin錛 X.錛 Ge錛 F.錛 Li錛 B. 2014. Cascade effects of crop species richness on the diversity of pest insects and their natural enemies. Science China Life Sciences 57: 718−725 Shi錛 P.錛 Chen錛 Z.錛 Yang錛 Q.錛 Harris錛 M.K.錛 Xiao錛 M. 2014. Influence of air temperature on the first flowering date of Prunusy edoensis Matsum. Ecology and Evolution 4: 292−299 Shi錛 P.J.錛 Zhao錛 Z.H.錛 Sandhu錛 H.S.錛 Hui錛 C.錛 Men錛 X.Y.錛 Ge錛 F.錛 Li錛 B.L. 2014. An optimization approach to the two-circle method of estimating ground-dwelling arthropod densities. Florida Entomologist 97: 644−6522015 Cheng錛 X.F.錛 Shi錛 P. (通信作者)錛 Hui錛 C.錛 Wang錛 F.S.錛 Liu錛 G.H.錛 Li錛 B.L. 2015. An optimal proportion of mixing broad-leaved forest for enhancing the effective productivity of moso bamboo. Ecology and Evolution 5: 1576−1584 Lu錛 Z.B.錛 Shi錛 P.J.錛 Reddy錛 G.V.P.錛 Li錛 L.M.錛 Men錛 X.Y.錛 Ge錛 F. 2015. Nonparametric estimation of interspecific spatio-temporal niche separation between two lady beetles (Coleoptera: Coccinellidae) in Bt cotton fields. Annals of the Entomological Society of America 108: 807−813 Reddy錛 G.V.P.錛 Shi錛 P.錛 Hui錛 C.錛 Cheng錛 X.錛 Ouyang錛 F.錛 Ge錛 F. 2015. The seesaw effect of winter temperature change on the recruitment of cotton bollworms Helicoverpa armigera through mismatched phenology. Ecology and Evolution 5: 5652−5661 Shi錛 P.J.錛 Huang錛 J.G.錛 Hui錛 C.錛 Grissino-Mayer錛 H.D.錛 Tardif錛 J.錛 Zhai錛 L.H.錛 Wang錛 F.S錛 Li錛 B.L. 2015. Capturing spiral radial growth of conifers using the superellipse to model tree-ring geometric shape. Frontiers in Plant Science 6: 856Shi錛 P.J.錛 Xu錛 Q.錛 Sandhu錛 H.S.錛 Gielis錛 J.錛 Ding錛 Y.L.錛 Li錛 H.R.錛 Dong錛 X.B. 2015. Comparison of dwarf bamboos (Indocalamus sp.) leaf parameters to determine relationship between spatial density of plants and total leaf area per plant. Ecology and Evolution 5: 4578−4589 2016 Liu錛 G.H.錛 Shi錛 P.J. (共同第一作者)錛 Xu錛 Q.錛 Dong錛 X.錛 Wang錛 F.S.錛 Wang錛 G.錛 Hui錛 C. 2016. Does the size-density relationship developed for bamboo species conform to the self-thinning rule? Forest Ecology and Management 361: 339−345 Ouyang錛 F.錛 Hui錛 C.錛 Men錛 X.錛 Zhang錛 Y.錛 Fan錛 L.錛 Shi錛 P.錛 Zhao錛 Z.錛 Ge錛 F. 2016. Early eclosion of overwintering cotton bollworm moths from warming temperatures accentuates yield loss in wheat. Agriculture錛 Ecosystems and Environment 217: 89−98 Shi錛 P.J.錛 Chen錛 L.錛 Hui錛 C.錛 Grissino-Mayer錛 H.D. 2016. Capture the time when plants reach their maximum body size by using the beta sigmoid growth equation. Ecological Modelling 320: 177−181 Shi錛 P.J.錛 Reddy錛 G.V.P.錛 Chen錛 L.錛 Ge錛 F. 2016. Comparison of thermal performance equations in describing temperature-dependent developmental rates of insects: (I) empirical models. Annals of the Entomological Society of America 109: 211−215 Shi錛 P.J.錛 Wei錛 J.Z.錛 Sandhu錛 H.S.錛 Liang錛 G.M. 2016. Capture the interaction types of two Bt toxins Cry1Ac and Cry2Ab on suppressing the cotton bollworm by using the multi-exponential equations. Insect Science 23: 649−654 Chen錛 L.錛 Li錛 Z.B.錛 Hui錛 C.錛 Cheng錛 X.錛 Li錛 B.L.錛 Shi錛 P. (通信作者) 2016. A general method for parameter estimation in light-response models. Scientific Reports 6: 27905Shi錛 P.J.錛 Sandhu錛 H.S.錛 Reddy錛 G.V.P. 2016. Dispersal distance determines the exponent of the spatial Taylor’s power law. Ecological Modelling 335: 48−53 Pan錛 Y.錛 Bai錛 B.錛 Xiong錛 T.錛 Shi錛 P.錛 Lu錛 C. 2016. Seed handling by primary frugivores differentially influence post-dispersal seed removal of Chinese yew by ground-dwelling animals. Integrative Zoology 11: 191−198 Lin錛 S.錛 Zhang錛 L.錛 Reddy錛 G.V.P.錛 Hui錛 C.錛 Gielis錛 J.錛 Ding錛 Y.錛 Shi錛 P. (通信作者) 2016. A geometrical model for testing bilateral symmetry of bamboo leaf with a simplified Gielis equation. Ecology and Evolution 6: 6798−6806 Shi錛 P. 2016. Peer review report 2 on “Drought explains variation in the radial growth of white spruce in western Canada”. Agricultural and Forest Meteorology 217: 536 2017 Wei錛 Q.錛 Jiao錛 C.錛 Guo錛 L.錛 Ding錛 Y.錛 Cao錛 J.錛 Feng錛 J.錛 Dong錛 X.錛 Mao錛 L.錛 Sun錛 H.錛 Yu錛 F.錛 Yang錛 G.錛Shi錛 P.錛 Ren錛 G.錛 Fei錛 Z. 2017. Exploring key cellular processes and candidate genes regulating the primary thickening growth of Moso underground shoots. New Phyotologist 214: 81−96 Shi錛 P.J.錛 Reddy錛 G.V.P.錛 Chen錛 L.錛 Ge錛 F. 2017. Comparison of thermal performance equations in describing temperature-dependent developmental rates of insects: (II) Two thermodynamic models. Annals of the Entomological Society of America 110: 113−120 Shi錛 P.J.錛 Fan錛 M.L.錛 Ratkowsky錛 D.A.錛 Huang錛 J.G.錛 Wu錛 H.I錛 Chen錛 L.錛 Fang錛 S.Y.錛 Zhang錛 C.X. 2017. Comparison of two ontogenetic growth equations for animals and plants. Ecological Modelling 349: 1−10 Shi錛 P.錛 Chen錛 Z.錛 Reddy錛 G.V.P.錛 Hui錛 C.錛 Huang錛 J.錛 Xiao錛 M. 2017. 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